How to setup Outlook to send from an alias in Office 365 This will give you the ability to select the alias using the “From” button when composing a new email. There are two workarounds to this, the first is to use a distribution group and assign users permissions to send from that distribution group. The second, which is the method documented in this post is to set-up a second mail account within Outlook and use the account to send mail via the Office 365 SMTP servers. Although it is possible to assign many email aliases to a single account in Office 365 it is not easy to send as an alias using Outlook when composing a new email.
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